Advective Removal of Intraparticle Uranium from Contaminated Vadose Zone Sediments, Hanford, U.S.
نویسندگان
چکیده
منابع مشابه
Advective removal of intraparticle uranium from contaminated vadose zone sediments, Hanford, U.S.
A column study on U(VI)-contaminated vadose zone sediments from the Hanford Site, WA, was performed to investigate U(VI) release kinetics with water advection and variable geochemical conditions. The sediments were collected from an area adjacent to and below tank BX-102 that was contaminated as a result of a radioactive tank waste overfill event. The primary reservoir for U(VI) in the sediment...
متن کاملSpectroscopic and diffraction study of uranium speciation in contaminated vadose zone sediments from the Hanford site, Washington state.
Contamination of vadose zone sediments under tank BX-102 at the Hanford site, Washington, resulted from the accidental release of 7-8 metric tons of uranium dissolved in caustic aqueous sludge in 1951. We have applied synchrotron-based X-ray spectroscopic and diffraction techniques to characterize the speciation of uranium in samples of these contaminated sediments. UIII-edge X-ray absorption f...
متن کاملSpectroscopic evidence for uranium bearing precipitates in vadose zone sediments at the Hanford 300-area site.
Uranium (U) solid-state speciation in vadose zone sediments collected beneath the former North Process Pond (NPP) in the 300 Area of the Hanford site (Washington) was investigated using multi-scale techniques. In 30 day batch experiments, only a small fraction of total U (approximately 7.4%) was released to artificial groundwater solutions equilibrated with 1% pCO2. Synchrotron-based micro-X-ra...
متن کاملHanford Site Vadose Zone Studies: An Overview
899 The Hanford Site is 1517 km2 (586 mi2) in size, located in a sparsely populated area in the rain shadow of the Cascade Mountains, adjacent to the Columbia River in southeastern Washington State (Fig. 1). The Hanford Site was set aside in the early 1940s by the U.S. Government to perform a top-secret mission, the Manhattan Project, for production of plutonium for atomic weapons used to end W...
متن کاملGeomicrobiology of high-level nuclear waste-contaminated vadose sediments at the hanford site, washington state.
Sediments from a high-level nuclear waste plume were collected as part of investigations to evaluate the potential fate and migration of contaminants in the subsurface. The plume originated from a leak that occurred in 1962 from a waste tank consisting of high concentrations of alkali, nitrate, aluminate, Cr(VI), (137)Cs, and (99)Tc. Investigations were initiated to determine the distribution o...
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ژورنال
عنوان ژورنال: Environmental Science & Technology
سال: 2008
ISSN: 0013-936X,1520-5851
DOI: 10.1021/es071113m